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Obituary
Yoshito Kishi (1937-2023)
Yoshito Kishi (1937-2023)
Professor. Yoshito Kishi,
a member of the Honorary Editorial Associates of HETEROCYCLES,
has passed away on January 9, 2023 at the age of 85.
I deeply express my regret over his death.
Kunio Ogasawara
Editor
January 13, 2023
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Note | Regular issue | Vol 51, No. 8, 1999, pp.1945-1948
Published online, 1st January, 1970■ Selective Electrocatalytic Oxidation of Primary and Secondary Alcohols Mediated by Decahydroquinolinyl-N-oxyl Radical
Published online, 1st January, 1970
DOI: 10.3987/COM-99-8600
■ Selective Electrocatalytic Oxidation of Primary and Secondary Alcohols Mediated by Decahydroquinolinyl-N-oxyl Radical
Yoshitomo Kashiwagi,* Futoshi Kurashima, Jun-ichi Anzai, and Tetsuo Osa
*Graduate School of Pharmaceutical Sciences, Tohoku University, Aramaki, Aoba-ku, sendai 980-8578, Japan
Abstract
(±)-cis,cis4-Benzoyloxy-2,2,8a-trimethyldecahydroquinolinyl-N-oxyl reveals a reversible redox peak whose oxidation potential is at + 0.67 V vs. Ag/AgCl. The compound catalyzed the selective oxidation reactions of primary and secondry alcohols to aldehydes and ketones, respectively, in high current efficiency (86.4-92.7 %) and selectivity (100 %).
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